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Nitrate removal to its fate in wetland mesocosm filled with sponge iron: Impact of influent COD/N ratio

Zhihao Si, Xinshan Song, Xin Cao, Yuhui Wang, Yifei Wang, Yufeng Zhao, Xiaoyan Ge, Awet Arefe Tesfahunegn

《环境科学与工程前沿（英文）》 2020年 第14卷 第1期 doi: 10.1007/s11783-019-1183-7

摘要： CW-Fe allowed a high-performance of NO3‒-N removal at the COD/N ratio of 0. Higher COD/N resulted in lower chem-denitrification and higher bio-denitrification. The application of s-Fe0 contributed to TIN removal in wetland mesocosm. s-Fe0 changed the main denitrifiers in wetland mesocosm. Sponge iron (s-Fe0) is a porous metal with the potential to be an electron donor for denitrification. This study aims to evaluate the feasibility of using s-Fe0 as the substrate of wetland mesocosms. Here, wetland mesocosms with the addition of s-Fe0 particles (CW-Fe) and a blank control group (CW-CK) were established. The NO3‒-N reduction property and water quality parameters (pH, DO, and ORP) were examined at three COD/N ratios (0, 5, and 10). Results showed that the NO3‒-N removal efficiencies were significantly increased by 6.6 to 58.9% in the presence of s-Fe0. NH4+-N was mainly produced by chemical denitrification, and approximately 50% of the NO3‒-N was reduced to NH4+-N, at the COD/ratio of 0. An increase of the influent COD/N ratio resulted in lower chemical denitrification and higher bio-denitrification. Although chemical denitrification mediated by s-Fe0 led to an accumulation of NH4+-N at COD/N ratios of 0 and 5, the TIN removal efficiencies increased by 4.5%‒12.4%. Moreover, the effluent pH, DO, and ORP values showed a significant negative correlation with total Fe and Fe (II) (P<0.01). High-throughput sequencing analysis indicated that Trichococcus (77.2%) was the most abundant microorganism in the CW-Fe mesocosm, while Thauera, Zoogloea, and Herbaspirillum were the primary denitrifying bacteria. The denitrifiers, Simplicispira, Dechloromonas, and Denitratisoma, were the dominant bacteria for CW-CK. This study provides a valuable method and an improved understanding of NO3‒-N reduction characteristics of s-Fe0 in a wetland mesocosm.

关键词： Sponge iron     Wetland mesocosm     Electronic donor     Denitrification     COD/N ratio    

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The development of roadside green swales in the Chinese Sponge City Program: Challenges and opportunities

《工程管理前沿（英文）》   页码 566-581 doi: 10.1007/s42524-023-0267-z

摘要： Roadside green swales have emerged as popular stormwater management infrastructure in urban areas, serving to mitigate stormwater pollution and reduce urban surface water discharge. However, there is a limited understanding of the various types, structures, and functions of swales, as well as the potential challenges they may face in the future. In recent years, China has witnessed a surge in the adoption of roadside green swales, especially as part of the prestigious Sponge City Program (SCP). These green swales play a crucial role in controlling stormwater pollution and conserving urban water resources by effectively removing runoff pollutants, including suspended solids, nitrogen, and phosphorus. This review critically examines recent research findings, identifies key knowledge gaps, and presents future recommendations for designing green swales for effective stormwater management, with a particular emphasis on ongoing major Chinese infrastructure projects. Despite the growing global interest in bioswales and their significance in urban development, China’s current classification of such features lacks a clear definition or specific consideration of bioswales. Furthermore, policymakers have often underestimated the adverse environmental effects of road networks, as reflected in existing laws and planning documents. This review argues that the construction and maintenance of roadside green swales should be primarily based on three critical factors: Well-thought-out road planning, suitable construction conditions, and sustainable long-term funding. The integration of quantitative environmental standards into road planning is essential to effectively address the challenge of pollution from rainfall runoff. To combat pollution associated with roads, a comprehensive assessment of potential pollution loadings should be carried out, guiding the appropriate design and construction of green swales, with a particular focus on addressing the phenomenon of first flush. One of the major challenges faced in sustaining funds for ongoing maintenance after swale construction. To address this issue, the implementation of a green finance platform is proposed. Such a platform would help ensure the availability of funds for continuous maintenance, thus maximizing the long-term effectiveness of green swales in stormwater management. Ultimately, the findings of this review aim to assist municipal governments in enhancing and implementing future urban road designs and SCP developments, incorporating effective green swale strategies.

关键词： grass swale     infiltration swale     bioswale     wet swale     sponge city    

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Preparation and properties of a silver particle-coated and 1-dodecanethiol-modified superhydrophobic melamine sponge

《化学科学与工程前沿（英文）》 2022年 第16卷 第8期   页码 1237-1246 doi: 10.1007/s11705-022-2140-8

摘要： A Ag particle-coated and 1-dodecanethiol-modified melamine sponge (Ag-DDT-MS) was prepared through surface roughness by coating silver particles and subsequent grafting of a hydrophobic long hydrocarbon chain. Superhydrophobic and 3D porous Ag-DDT-MS was characterized by Fourier transform infrared spectroscopy, scanning electron microscope, energy-dispersive X-ray spectroscopy, and X-ray diffraction. The water contact angle of Ag-DDT-MS reached 159.2°. Ag-DDT-MS exhibited excellent absorption capacity for high viscous oils and organic solvents, ranging from 42.8 to 105.2 g∙g−1. The absorbed oils can be easily collected by the mechanical pressing process, and the oil recovery rate was satisfactory, more than 90% after 20 recycles. Ag-DDT-MS material also demonstrated good stability and excellent compression-recovery ability, keeping 88.6% of the initial height after ten compression-release cycles.

关键词： melamine sponge     oil-absorbing material     hydrophobic     oil-water separation     oil absorption capacity    

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Superhydrophobic, mechanically flexible and recyclable reduced graphene oxide wrapped sponge for highly

Lijuan Qiu, Ruiyang Zhang, Ying Zhang, Chengjin Li, Qian Zhang, Ying Zhou

《化学科学与工程前沿（英文）》 2018年 第12卷 第3期   页码 390-399 doi: 10.1007/s11705-018-1751-6

摘要：

Water pollution has become an urgent issue for our modern society, and it is highly desirable to rapidly deal with the water pollution without secondary pollution. In this paper, we have prepared a reduced graphene oxide (RGO) wrapped sponge with superhydrophobicity and mechanically flexibility via a facile low-temperature thermal treatment method under a reducing atmosphere. The skeleton of this sponge is completely covered with RGO layers which are closely linked to the skeleton. This sponge has an abundant pore structure, high selectivity, good recyclability, low cost, and outstanding adsorption capacity for floating oil or heavy oil underwater. In addition, this sponge can maintain excellent adsorption performance for various oils and organic solvents over 50 cycles by squeezing, and exhibits extremely high separation efficiencies, up to 6 × 106 and 3.6 × 106 L·m−3·h−1 in non-turbulent and turbulent water/oil systems, respectively. This superhydrophobic adsorbent with attractive properties may find various applications, especially in large-scale removal of organic contaminants and oil spill cleanup.

关键词： superhydrophobicity     mechanically flexibility     water/oil separation     reduced graphene oxide wrapped sponge    

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China’s Sponge City construction: A discussion on technical approaches

Haifeng Jia, Zheng Wang, Xiaoyue Zhen, Mike Clar, Shaw L. Yu

《环境科学与工程前沿（英文）》 2017年 第11卷 第4期 doi: 10.1007/s11783-017-0984-9

摘要： Since 2014, China has been implementing the Sponge City Construction initiative, which represents an enormous and unprecedented effort by any government in the world for achieving urban sustainability. According to preliminary estimates, the total investment on the Sponge City Plan is roughly 100 to 150 million Yuan (RMB) ($15 to $22.5 million) average per square kilometer or 10 Trillion Yuan (RMB) ($1.5 Trillion) for the 657 cities nationwide. The Sponge City Plan (SCP) calls for the use of natural processes such as soil and vegetation as part of the urban runoff control strategy, which is similar to that of low impact development (LID) and green infrastructure (GI) practices being promoted in many parts of the world. The SCP includes as its goals not only effective urban flood control, but also rainwater harvest, water quality improvement and ecological restoration. So far, the SCP implementation has encountered some barriers and challenges due to many factors. The present paper presents a review of those barriers and challenges, offers discussions and recommendations on several technical aspects such as control goals and objectives; planning/design and construction of LID/GI practices; performance evaluation. Several key recommendations are proposed on Sponge City implementation strategy, Site-specific regulatory framework and technical guidance, Product innovation and certification, LID/GI Project financing, LID/GI professional training and certification, public outreach and education. It is expected that the successful implementation of the SCP not only will bring about a sustainable, eco-friendly urbanization process in China, but also contribute enormously to the LID/GI research and development with the vast amount of relevant data and experiences generated from the Sponge City construction projects.

关键词： Low impact development (LID)     Green infrastructure (GI)     Sponge City     Barriers     Construction strategies    

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Low Impact Development and Sponge City Construction for Urban Stormwater Management

Haifeng Jia, Shaw L. Yu, Huapeng Qin

《环境科学与工程前沿（英文）》 2017年 第11卷 第4期 doi: 10.1007/s11783-017-0989-4

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Upgrading to urban water system 3.0 through sponge city construction

Nanqi Ren, Qian Wang, Qiuru Wang, Hong Huang, Xiuheng Wang

《环境科学与工程前沿（英文）》 2017年 第11卷 第4期 doi: 10.1007/s11783-017-0960-4

摘要： Urban water system 3.0 (Blue, gray, brown and yellow arrows represent water flow, wastewater flow, resource and energy respectively) Facing the pressure of excessive water consumption, high pollution load and rainstorm waterlogging, linear and centralized urban water system, system 2.0, as well as traditional governance measures gradually exposed characters of water-sensitivity, vulnerability and unsustainability, subsequently resulting in a full-blown crisis of water shortage, water pollution and waterlogging. To systematically relieve such crisis, we established healthy urban water-cycling system 3.0, in which decentralized sewerage systems, spongy infrastructures and ecological rivers play critical roles. Through unconventional water resource recycling, whole process control of pollutions and ecological restoration, system 3.0 with integrated management measures, is expected to fit for multiple purposes which involve environmental, ecological, economic and social benefits. With advantages of flexibility, resilience and sustainability, water system 3.0 will show an increasingly powerful vitality in the near future.

关键词： Water crisis     Urban water system     Spongy city     Decentralized system     Multi-purpose    

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reduction of chromium(VI) to chromium(III) using nitrogen-doped porous carbon adsorbent derived from loofah sponge

《环境科学与工程前沿（英文）》 2022年 第16卷 第5期 doi: 10.1007/s11783-021-1491-6

摘要：

• A high-efficiency N-doped porous carbon adsorbent for Cr(VI) was synthesized.

关键词： Chromium(VI)     Nitrogen-doped porous carbon     Adsorption     Reduction     Loofah sponge    

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randomized, controlled, open label non-inferiority trial of intravenous ferric carboxymaltose versus ironsucrose in patients with iron deficiency anemia in China

《医学前沿（英文）》 doi: 10.1007/s11684-023-1001-2

摘要： Iron deficiency (ID) and ID anemia (IDA) pose significant public health concerns in China. Although iron sucrose (IS) treatment is well-established in the country, ferric carboxymaltose (FCM) offers the advantage of higher doses and fewer infusions. This open label, randomized, controlled, non-inferiority trial was conducted at multiple sites in China to compare the outcomes of FCM (maximum of 2 doses, 500 or 1000 mg iron) and IS (up to 11 infusions, 200 mg iron) treatments in subjects with IDA. The primary endpoint was the achievement of hemoglobin (Hb) response (an increase of ≥2 g/dL from baseline) within 8 weeks, whereas secondary endpoints included changes in Hb, transferrin saturation, and serum ferritin levels. Among the 371 randomized subjects, a similar percentage of subjects treated with FCM and IS achieved Hb-response (FCM 99.4%, IS 98.3%), thereby confirming the non-inferiority of FCM compared with IS (difference 1.12 (−2.15, 4.71; 95% confidence interval (CI))). Furthermore, a significantly higher proportion of FCM-treated subjects achieved early Hb-response at Week 2 (FCM 85.2%, IS 73.2%; difference 12.1 (3.31, 20.65; 95% CI)). Additionally, the increase in TSAT and serum ferritin levels from baseline was significantly greater at all time points for FCM-treated subjects. The safety profiles of FCM and IS were comparable, with the exception of transient hypophosphatemia and pyrexia, which are consistent with FCM’s known safety profile. In conclusion, FCM proves to be an efficacious treatment for IDA, providing faster Hb-response and correction of ID with fewer administrations than IS.

关键词： iron deficiency     anemia     intravenous iron     ferric carboxymaltose     iron sucrose     Hb response     early response    

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Synergistic effects of sodium hypochlorite disinfection and iron-oxidizing bacteria on early corrosionin cast iron pipes

《环境科学与工程前沿（英文）》 2022年 第16卷 第6期 doi: 10.1007/s11783-021-1506-3

摘要：

• The early corrosion process in the cast iron pipes was investigated.

关键词： Cast iron pipe corrosion     Drinking water distribution systems     Chlorine disinfection     Iron-oxidizing bacteria     Coupling effects    

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Performance of iron-air battery with iron nanoparticle-encapsulated C–N composite electrode

《能源前沿（英文）》 doi: 10.1007/s11708-023-0913-5

摘要： Highly efficient and stable iron electrodes are of great significant to the development of iron-air battery (IAB). In this paper, iron nanoparticle-encapsulated C–N composite (NanoFe@CN) was synthesized by pyrolysis using polyaniline as the C–N source. Electrochemical performance of the NanoFe@CN in different electrolytes (alkaline, neutral, and quasi-neutral) was investigated via cyclic voltammetry (CV). The IAB was assembled with NanoFe@CN as the anode and IrO2 + Pt/C as the cathode. The effects of different discharging/charging current densities and electrolytes on the battery performance were also studied. Neutral K2SO4 electrolyte can effectively suppress the passivation of iron electrode, and the battery showed a good cycling stability during 180 charging/discharging cycles. Compared to the pure nano-iron (NanoFe) battery, the NanoFe@CN battery has a more stable cycling stability either in KOH or NH4Cl + KCl electrolyte.

关键词： energy storage and conversion     metallic composites     nanocomposites     iron-air battery     iron anode    

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Redox reactions of iron and manganese oxides in complex systems

Jianzhi Huang, Huichun Zhang

《环境科学与工程前沿（英文）》 2020年 第14卷 第5期 doi: 10.1007/s11783-020-1255-8

摘要： • Mechanisms of redox reactions of Fe- and Mn-oxides were discussed. • Oxidative reactions of Mn- and Fe-oxides in complex systems were reviewed. • Reductive reaction of Fe(II)/iron oxides in complex systems was examined. • Future research on examining the redox reactivity in complex systems was suggested. Conspectus Redox reactions of Fe- and Mn-oxides play important roles in the fate and transformation of many contaminants in natural environments. Due to experimental and analytical challenges associated with complex environments, there has been a limited understanding of the reaction kinetics and mechanisms in actual environmental systems, and most of the studies so far have only focused on simple model systems. To bridge the gap between simple model systems and complex environmental systems, it is necessary to increase the complexity of model systems and examine both the involved interaction mechanisms and how the interactions affected contaminant transformation. In this Account, we primarily focused on (1) the oxidative reactivity of Mn- and Fe-oxides and (2) the reductive reactivity of Fe(II)/iron oxides in complex model systems toward contaminant degradation. The effects of common metal ions such as Mn2+ , Ca2+, Ni2+, Cr3+ and Cu2+, ligands such as small anionic ligands and natural organic matter (NOM), and second metal oxides such as Al, Si and Ti oxides on the redox reactivity of the systems are briefly summarized.

关键词： Iron oxides     manganese oxides     reduction     oxidation     complex systems     reaction kinetics and mechanisms    

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Mechanical properties of vanadium-alloyed austempered ductile iron for crankshaft applications

《机械工程前沿（英文）》 2023年 第18卷 第3期 doi: 10.1007/s11465-023-0746-2

摘要： This study focused on the development of austempered ductile iron (ADI) with desirable combination of mechanical properties for crankshaft applications by the combined effect of vanadium (V) alloying and an optimized heat treatment process. The produced unalloyed GGG60, 0.15% V-alloyed GGG60 (V-15), and 0.30% V-alloyed GGG60 samples were subjected to austenitizing at 900 °C for 1 h and subsequent austempering processes at 250, 300, and 350 °C for 15, 30, 60, 90, and 180 min. As a result of these austempering processes, different bainitic structures were obtained, which led to the formation of diverse combinations of mechanical properties. The mechanical properties of the austempered samples were tested comprehensively, and the results were correlated with their microstructures and the stability of the retained austenite phases. From the microstructural observations, the V-alloyed samples exhibited a finer microstructure and a more acicular ferrite phase than unalloyed samples. The V addition delayed the coarsening of the acicular ferrite structures and considerably contributed to the improvement of the mechanical properties of GGG60. Moreover, the X-ray diffraction results revealed that the retained austenite volume and the carbon enrichment of austenite phases in ADI samples were remarkably affected by the addition of vanadium. The increase in volume fraction of retained austenite and its carbon content provided favorable ductility and toughness to V-15, as confirmed by the elongation and impact test results. Consequently, the dual-phase ausferrite microstructure of V-15 that was austempered at 300 °C for 60 min exhibited high strength with substantial ductility and toughness for crankshaft applications.

关键词： austempered ductile iron (ADI)     vanadium alloying     mechanical properties     crankshafts     retained austenite    

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Scrap Iron Filings assisted nitrate and phosphate removal in low C/N waters using mixed microbial culture

《环境科学与工程前沿（英文）》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1358-2

摘要：

• Microbes enhance denitrification under varying DO concentrations and SIF dosages.

关键词： Scrap iron filing     Nitrate removal     Phosphate removal     Mixed culture denitrification     Zero valent iron    

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Highly selective and green recovery of lithium ions from lithium iron phosphate powders with ozone

《化学科学与工程前沿（英文）》 2023年 第17卷 第6期   页码 749-758 doi: 10.1007/s11705-022-2261-0

摘要： Since lithium iron phosphate cathode material does not contain high-value metals other than lithium, it is therefore necessary to strike a balance between recovery efficiency and economic benefits in the recycling of waste lithium iron phosphate cathode materials. Here, we describe a selective recovery process that can achieve economically efficient recovery and an acceptable lithium leaching yield. Adjusting the acid concentration and amount of oxidant enables selective recovery of lithium ions. Iron is retained in the leaching residue as iron phosphate, which is easy to recycle. The effects of factors such as acid concentration, acid dosage, amount of oxidant, and reaction temperature on the leaching of lithium and iron are comprehensively explored, and the mechanism of selective leaching is clarified. This process greatly reduces the cost of processing equipment and chemicals. This increases the potential industrial use of this process and enables the green and efficient recycling of waste lithium iron phosphate cathode materials in the future.

关键词： lithium iron phosphate powder     stoichiometric number     selective leaching     lithium recovery    

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标题 作者 时间 类型 操作

Nitrate removal to its fate in wetland mesocosm filled with sponge iron: Impact of influent COD/N ratio

Zhihao Si, Xinshan Song, Xin Cao, Yuhui Wang, Yifei Wang, Yufeng Zhao, Xiaoyan Ge, Awet Arefe Tesfahunegn

期刊论文

The development of roadside green swales in the Chinese Sponge City Program: Challenges and opportunities

期刊论文

Preparation and properties of a silver particle-coated and 1-dodecanethiol-modified superhydrophobic melamine sponge

期刊论文

Superhydrophobic, mechanically flexible and recyclable reduced graphene oxide wrapped sponge for highly

Lijuan Qiu, Ruiyang Zhang, Ying Zhang, Chengjin Li, Qian Zhang, Ying Zhou

期刊论文

China’s Sponge City construction: A discussion on technical approaches

Haifeng Jia, Zheng Wang, Xiaoyue Zhen, Mike Clar, Shaw L. Yu

期刊论文

Low Impact Development and Sponge City Construction for Urban Stormwater Management

Haifeng Jia, Shaw L. Yu, Huapeng Qin

期刊论文

Upgrading to urban water system 3.0 through sponge city construction

Nanqi Ren, Qian Wang, Qiuru Wang, Hong Huang, Xiuheng Wang

期刊论文

reduction of chromium(VI) to chromium(III) using nitrogen-doped porous carbon adsorbent derived from loofah sponge

期刊论文

randomized, controlled, open label non-inferiority trial of intravenous ferric carboxymaltose versus ironsucrose in patients with iron deficiency anemia in China

期刊论文

Synergistic effects of sodium hypochlorite disinfection and iron-oxidizing bacteria on early corrosionin cast iron pipes

期刊论文

Performance of iron-air battery with iron nanoparticle-encapsulated C–N composite electrode

期刊论文

Redox reactions of iron and manganese oxides in complex systems

Jianzhi Huang, Huichun Zhang

期刊论文

Mechanical properties of vanadium-alloyed austempered ductile iron for crankshaft applications

期刊论文

Scrap Iron Filings assisted nitrate and phosphate removal in low C/N waters using mixed microbial culture

期刊论文

Highly selective and green recovery of lithium ions from lithium iron phosphate powders with ozone

期刊论文